Digital Colloids: Reconfigurable Clusters as High Information Density Elements

TitleDigital Colloids: Reconfigurable Clusters as High Information Density Elements
Publication TypeJournal Article
Year of Publication2014
AuthorsPhillips, CL, Jankowski, E, Krishnatreya, BJ, Edmond, KV, Sacanna, S, Grier, DG, Pine, DJ, Glotzer, SC
JournalSoft Matter
Volume10
Pagination7468-7479
Date Published07/2014
Other NumbersANL/MCS-P5172-0714
AbstractThrough the design and manipulation of discrete, nanoscale systems capable of encoding massive amounts of information, the basic components of computation are open to reinvention. These components enable tagging, memory storage, and sensing in unusual environments – elementary functions crucial for soft robotics and “wet computing”. Here we show how reconfigurable clusters made of N colloidal particles bound flexibly to a central colloidal sphere have the capacity to store an amount of information that increases as O(N!). Using Brownian dynamics simulations, we predict dynamical regimes that allow for information to be written, saved, and erased. We experimentally assemble an N = 4 reconfigurable cluster from chemically synthesized colloidal building blocks, and monitor its equilibrium dynamics. We observe state switching in agreement with simulations. This cluster can store one bit of information, and represents the simplest digital colloid.  
DOI10.1039/C4SM00796D
PDFhttp://www.mcs.anl.gov/papers/P5172-0714.pdf